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It should be possible to build a surrogate over new outputs if they are extractable from previous surrogate save files, even if they weren't originally defined in surr.coupling_vars.
Actual Behavior
If you want the surrogate to predict a certain output, it must be defined with SystemSurrogate.coupling_vars up front, before training.
This means you cannot predict a new output without retraining a new SystemSurrogate, even if that output is already computed and saved to file.
Expected Behavior
surr.coupling_vars.Actual Behavior
SystemSurrogate.coupling_varsup front, before training.SystemSurrogate, even if that output is already computed and saved to file.